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TitleEnzymatic Birch reduction via hydrogen atom transfer at [4Fe-4S]-OH 2 and [8Fe-9S] clusters.
Journal, issue, pagesNat Commun, Vol. 16, Page 3236-3236, Year 2025
Publish dateFeb 13, 2024 (structure data deposition date)
AuthorsFuchs, J. / Fernandez-Arevalo, U. / Demmer, U. / Diaz, E. / Ullmann, G.M. / Pierik, A.J. / Ermler, U. / Boll, M.
External linksNat Commun / PubMed:40185728
MethodsX-ray diffraction
Resolution1.35 - 1.6 Å
Structure data

PDB-8s02:
BzdNO-benzoyl-CoA complex
Method: X-RAY DIFFRACTION / Resolution: 1.35 Å

PDB-8s1t:
BzdNO-cyclohexa-1,5-diene-1-carboxy-CoA complex
Method: X-RAY DIFFRACTION / Resolution: 1.45 Å

PDB-8s2r:
BzdNO in partially coenzyme A - free state
Method: X-RAY DIFFRACTION / Resolution: 1.6 Å

Chemicals

ChemComp-BYC:
benzoyl coenzyme A

ChemComp-GOL:
GLYCEROL

ChemComp-SF4:
IRON/SULFUR CLUSTER

ChemComp-BJ8:
Double cubane cluster

ChemComp-TRS:
2-AMINO-2-HYDROXYMETHYL-PROPANE-1,3-DIOL / pH buffer*YM

ChemComp-HOH:
WATER

ChemComp-4KX:
1,5 Dienoyl-CoA

Source
  • azoarcus sp. cib (bacteria)
KeywordsOXIDOREDUCTASE / Benzoyl-CoA reductase / reductive dearomatization / iron-sulfur clusters

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